ATLAS: Atomic Translation&Language for Automated Structures
Large language models struggle to directly generate atomic structures satisfying global physical constraints such as periodicity and bond lengths, as conventional token-by-token generation lacks physical plausibility. This work proposes ATLAS, a framework that leverages component algebra to translate natural language into verifiable structure-building scripts. By introducing a checklist-based verification scoring mechanism and a JSON-formatted construction engine, the framework enables deterministic replay, rendering the LLM translation process both measurable and controllable. ATLAS successfully demonstrates the generation of fourteen structural classes spanning crystalline to amorphous networks, and can be directly applied to constructing training datasets for machine learning force fields.